Evolution
A support site for modules SC0060-3 Evolution

and SCM009-M Molecular Evolution

Page last updated 11/02/02

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Prebiotic evolution
[required for SC0060-3 only]

Prebiotic evolution can be defined as the processes that led to the first living cells
(ie, the 'origin of life'; ie, evolution prior to life - hence 'prebiotic').
Prebiotic evolution is
a difficult topic for science, as very limited physical evidence remains, and there are a
number of considerable physical and chemical obstacles that had to be overcome.

The oldest fossils so far discovered are simple bacteria-like cells in stromatolites, which are rocky stratified
deposits laid down by microbes, eg, ca.3,500,000,000 year old fossilised stromatolites Western Australia.

The essential requirements for prebiotic evolution are:

A key problem is that the latter characteristics of a living cell are highly interdependent,
but it is most unlikely they all evolved at same time - ie, a 'chicken and egg' problem.

The universe is ca.15,000,000,000 years old, and was initially consisted of ca.75% Hydrogen and ca.25% Helium, and all heavier
nuclei formed from subsequent stellar nuclear fusion. Thus was life not
possible in the early universe until the requisite nuclei
(C, N, O, etc) were formed in stars, dispersed by
supernova explosions and then taken up into planets during new star formation.

Our sun formed ca.4,600,000,000 years ago, and Earth accreted from the heavier atoms.

It is possible to experimentally stimulate primordial Earth. An 'atmosphere' of water vapour, hydrogen, nitrogen, carbon monoxide,
carbon dioxide and perhaps hydrogen sulphide (all believed to have been present in the primordial atomsphere) is subjected to
energy sources such as ultraviolet radiation (ie, to simulate the sun), electrical discharges (to stimulate
lightning) and radioactivity
(both cosmic and terrestrial radiation were significant on primordial Earth).
Such 'Miller & Urey' experimental simulations have
produced all twenty of the biological amino acids (the building blocks of proteins) and
several others in an L/D racemic mix, and
also purine and pyrimidine bases (building blocks of nucleic acids like RNA and DNA), porphyrins (the ring structure found in
haemoglobin, myoglobin and cytochromes), a number of sugars, and some fatty acids.

The primordial atmosphere was 'reducing' in that there was no oxygen present. This is vital because otherwise any molecules
formed as above would have been rapidly oxidised (which is what would happen in the modern atmosphere of 21% oxygen).

The above experiments also produce much hydrogen cyanide (HCN) and formaldehyde (HCHO). This may be important because
5HCN can give the purine base adenine and nHCHO can give nC-sugar (eg, 5HCHO gives C5 pentoses, 6HCHO give C6 hexoses, etc)
under UV irradiation. Overall, it is
estimated that ca.3,000,000 tonnes of organic molecules were produced per year on young Earth,~
and with no oxygen or organisms to break them down, then lots will have
accumulated.

Another more recent idea is that comets impacting on primordial Earth brought alot of water and organic molecules. Comets certainly
are largely composed of water and are also rich in organic molecules, and the young Earth was intensively bomdarded by comets for
the first 1,000,000,000 years or so. In fact, some cosmologists believe most of the water on Earth is cometary!

Mechanisms are then required to join the above smaller building blocks together to form larger biological 'macromolecules'.
Amino acids join to form polypeptides/proteins, purine and pyrimidine bases join with sugars and phosphate to form
nucleic acids (like RNA and DNA), and fatty acids join with phosphate and other alcohols to form phospholipids which
then assemble to form the bilayer of biological membranes. An old idea for this is the 'primordial soup' concept where
organic molecules in aqueous solution condensed
to form macromolecules. However, a major problem with this is that
condensation is not a favourable reaction in aqueous solution - the macromolecules are more likely to break down!

A more recent and feasible idea is the 'primordial pizza' concept where organic molecules in dried and/or semi-dried
(gel) surface phases condensed to form macromolecules
. In such a state, the increased reactant concentrations and
decreased degrees of freedom
make condensation a much more favourable reaction. Primordial pizzas could have
risen from pools evaporated by the sun or volcanic activity, or between
the mineral stacks of clay. Clay consists of
thin mineral layers interspersed with thin water layers, and also contains potentially catalytic metal atoms.

Cairns-Smith proposed a key role for clay in prebiotic evolution, but his ideas have recently lost much credence.

Primordial pizzas have been experimentally stimulated. For example, anhydrous (water-free) mixtures of amino acids heated
at 120 oC for one week form polypeptides of
formula weight ca.20,000. These have been called 'proteinoids' by Fox, who has
been able to demostrate that they can show limited
enzyme activities. There is similar data for clays but at lower temperatures
and with water present.

The next stage must be aggregation of these macromolecules into larger (but not yet necessarily living) assemblies. There are a
number of possibilities. 'Coacervates' were discovered some time ago and are spontaneously formed droplets of polypeptides in
aqueous solution. These are stable, but rather too large with ca.500 micrometre
diameter. Fox more recently discovered
' microspheres', formed by heating then cooling of aqueous solution
of proteinoid (see above). These are stable, with a more
realistic ca.1-2 micron diameter, and comprise tiny volumes of water enclosed
within a boundary layer of polypeptide.
Micelles have long been known and are spherical bilayers of phospholipid spontaneously formed in aqueous solution.
Adsorption into interstices of clays could have provided a nurturing environ for the above kinds of aggregates.

Micelles may seem the best idea above, since modern biological membranes are phospholipid bilayers. However, membrane
bilayers require unbranched fatty acids of chain
length greater than ten carbons, but primordial processes only give branched
fatty acids of
less than ten carbon chain length. Microspheres may be promising, but the boundary layer is proteinoid not
phospholipid bilayer. At least the above experimental finding show what can be possible.

Research has now found that aggregates like those above can display some living characteristics such as uptake, retention and
concentration of external molecules
(so producing an internal environment different to the exterior), increase in size (through the
uptake of external molecules), 'division' (through mechanical shear after size increase),
and can be even subject to selection!

Nonetheless, aggregates are certainly not living. The most critical aspect absent is a system of heredity. Inheritance in aggregates
is limited to the 'sample' of internal molecules the two daughter aggregates receive from the splitting parent aggregate. This could,
of course, has been the first heredity system! The chicken and egg kind of problem is a major obstacle here, in that RNA/DNA
genes are required to produce
specific proteins, yet specific proteins are required to produce DNA/RNA!

A currently popular idea is that RNA was the first true genetic material (a notion known as the 'RNA World'). RNA is indeed
produced by primordial processes, whereas DNA is not, so RNA almost certainly prededed DNA. RNA can adopt

sequence-dependent 3D conformations like proteins do (eg, modern tRNAs and
rRNAs do this). RNA can give specific
catalytic activities like enzyme proteins do (eg, these 'ribozyme' activities exist in and are crucial to modern cells -
eg, intron splicing of pre-mRNAs is auto-catalysed by the RNA).
RNA can specifically bind amino acids (eg, modern tRNAs
do this).
Therefore, perhaps RNA preceded DNA and proteins, so solving the chicken and egg conumdrum. However, proteins
are formed in prebiotic processes, so this idea does not entirely satisfy.

Other ideas for the first true genetic material include polypeptides specifically catalysing their own formation - ie, proteins as
first genetic code! Perhaps some other molecule acted as the genetic code? Structural patterns in clay minerals
were suggested
by Cairns-Smith as a possible first genetic code. There is little evidence for any of these ideas, and the RNA world concept
currently holds sway.

Overall, abiotic (without life) formation of biological macromolecules and then aggregates seems both theoretically well
established and supported by
good experimental evidence. However, going from aggregates to living cells is less clear
and with not much experimental evidence so far.

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